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A new method for calculating the vibration-rotation-tunneling spectra of molecular clusters and its application to the water dimer

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A new method is developed for calculating the vibration-rotation-tunneling spectra of molecular clusters consisting of rigid monomers. The method is based on generation of optimized bases for each monomer. First, a sequential symmetry adaptation procedure is developed for relating the symmetries of monomer basis functions with the symmetries of the eigenstates of the cluster. Then this symmetry adaptation procedure is used in the generation of optimized bases and combining them for finding the eigenstates. |

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